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J Ivin and T Saegusa, eds, Elsevier, London, 1984 Goethals, E J, Cationic Ring-Opening Polymerization: Amines and N-Containing Heterocycles, Chap 52 in Comprehensive Polymer Science, Vol 3, G C Eastmond, A Ledwith, S Russo, and P Sigwalt, eds, Pergamon Press, London, 1989a Goethals, E J, Cationic Ring-Opening Polymerization: Sul des, Chap 51 in Comprehensive Polymer Science, Vol 3, G C Eastmond, A Ledwith, S Russo, and P Sigwalt, eds, Pergamon Press, London, 1989b Goethals, E J, M Dubreuil, Y Wang, I De Witte, D Christova, S Verbrugghe, N Yanul, L Tanghe, G Mynarczuk, and F Du Prez, Macromol Symp, 153, 209 (2000) Good, F J, Jr and C Schuerch, Macromolecules, 18, 595 (1985) Goodman, M, E Peggion, M Szwarc, and C H Bamford, Macromolecules, 10, 1299 (1977) Greene, R M E, K J Ivin, J J Rooney, J.

Kress, and J A Osborn, Makromol Chem, 189, 2797 (1988) Gross, R A, Y Zhang, G Konrad, and R W Lenz, Macromolecules, 21, 2657 (1988) Gross, R A, A Kumar, and B Kalra, Chem Rev, 101, 2097 (2001) Grubbs, R H, D A Dougherty, and T M Swager, J Am Chem Soc, 110, 2973 (1988) Gunatillake, P A, G Odian, and D A Tomalia, Macromolecules, 20, 2356 (1987); 21, 1556 (1988)..

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2-57

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The first thing that we note is that, unlike the single perceptron, the fitted values may approach any target values in the range ( 0 , l ) by varying the choice of and u l . Hence, for the multi-layer perceptron, i t does not appear unreasonable to have target values other than 0 and 1, and the common practice of using target values of 0.1 and 0.9 appears to have some vindication. In 9 (p. 143) we show that using target values of { O . l , 0.9) may give a smoother separating boundary; however, it also has the undesirable effect that the outputs at the qth output unit may no = klz) (see Section 4.2, p. 35). longer be simply interpreted as an estimate of More importantly for our discussion here, unless the values of the limits exactly

The inherent viscosity Zinh is a measure of the polymer molecular weight. Larger values of Zinh indicate higher molecular weights. Early precipitation of the polyurethane occurs in

TABLE 2-4 Effect of Solvent on Molecular Weight in Polymerization of Bis(4-isocyanatophenyl)methane with Ethylene Glycola; b Solvent Xylene Chlorobenzene Nitrobenzene Dimethyl sulfoxide Zc inh 0.06 0.17 0.36 0.69 Solubility of Polymer Precipitates at once Precipitates at once Precipitates after 1 h 2 Polymer is soluble

a Data from Lyman [1960]. b Polymerization temperature: 115 C. c Measured in dimethylformamide at room temperature.

Figure 8.4 The shape the ICs for the R weights for an MLP with a hidden layer. The IC, given as dotted lines, should be interpreted as a surface sitting over the page. In a direction not parallel to the decision hyperplane, the IC redescends to 0. In a direction parallel to the decision hyperplane, it is unbounded. There are two exceptions to this. One is the IC for the bias term, which is constant along paths parallel to the decision boundary. The ot,her is the IC,,,, when the decision boundary is perpendicular to the axis. In this case also the IC takes a constant value along paths parallel to the decision boundary.

xylene and chlorobenzene and limits the polymerization to a low molecular weight. Higher molecular weights are obtained when the solvent for the reaction becomes a better solvent for the polymer. The highest polymer molecular weight is obtained in DMSO (dimethylsulfoxide), a highly polar aprotic solvent, in which the polyurethane is completely soluble during the entire course of the polymerization. Figure 2-7 shows similar behavior for the polymerization between terephthaloyl chloride and trans-2,5-dimethylpiperazine in mixtures of chloroform with carbon tetrachloride or

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Fig. 2-7 Polymerization of terephthaloyl chloride and trans-2,5-dimethylpiperazine in mixed solvents. After Morgan [1963, 1965] (by permission of Wiley-Interscience, New York).

n-hexane [Morgan, 1963, 1965] Chloroform is a good solvent for the polymer, while carbon tetrachloride and n-hexane are poor solvents The inherent viscosity of the polymer (measured at 30 C in m-cresol) increases as the reaction mixture contains a larger proportion of chloroform The better the reaction medium as a solvent for the polymer the longer the polymer stays in solution and the larger the polymer molecular weight With a solvent medium that is a poor solvent for polymer, the molecular weight is limited by precipitation Other examples of this behavior are described in Secs 2-8c and 2-14.

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